高等学校化学学报 ›› 2022, Vol. 43 ›› Issue (9): 20220347.doi: 10.7503/cjcu20220347

• 展望 • 上一篇    下一篇

单原子材料在二氧化碳催化中的技术经济分析与产业化应用前景

王新天2, 李攀2, 曹越1, 洪文浩2, 耿忠璇2, 安志洋2, 王昊宇2, 王桦3, 孙斌1(), 朱文磊2(), 周旸1()   

  1. 1.南京邮电大学有机电子与信息显示国家重点实验室和先进材料研究院, 南京 210023
    2.污染控制与资源化研究国家重点实验室, 生命分析化学国家重点实验室, 关键地球物质循环前沿科学中心, 南京大学环境学院, 化学化工学院, 南京 210023
    3.湖州师范学院生命科学学院, 湖州 313000
  • 收稿日期:2022-05-16 出版日期:2022-09-10 发布日期:2022-07-28
  • 通讯作者: 孙斌,朱文磊,周旸 E-mail:iambsun@njupt.edu.cn;wenleizhu@nju.edu.cn;iamyangzhou@njupt.edu.cn
  • 基金资助:
    国家自然科学基金(22176086);江苏省自然科学基金(BK20210189);江苏省自然科学基金青年项目(SBK2022044384);南京邮电大学科研启动基金(NY221005);南京大学污染控制与资源化研究国家重点实验室基金(PCRR-ZZ-202106);中央高校基本科研业务费专项资金(021114380183);南京大学关键地球物质循环前沿科学中心研究经费和江苏省特聘教授研究经费(RK030STP21007)

Techno-economic Analysis and Industrial Application Prospects of Single-atom Materials in CO2 Catalysis

WANG Xintian2, LI Pan2, CAO Yue1, HONG Wenhao2, GENG Zhongxuan2, AN Zhiyang2, WANG Haoyu2, WANG Hua3, SUN Bin1(), ZHU Wenlei2(), ZHOU Yang1()   

  1. 1.State Key Laboratory for Organic Electronics and Information Displays & Institute of Advanced Materials(IAM),Nanjing University of Posts & Telecommunications,Nanjing 210023,China
    2.State Key Laboratory of Pollution Control and Resource Reuse,State Key Laboratory of Analytical Chemistry for Life Science,the Frontiers Science Center for Critical Earth Material Cycling,School of the Environment,School of Chemistry and Chemical Engineering,Nanjing University,Nanjing 210023,China
    3.School of Life Sciences,Huzhou University,Huzhou 313000,China
  • Received:2022-05-16 Online:2022-09-10 Published:2022-07-28
  • Contact: SUN Bin,ZHU Wenlei,ZHOU Yang E-mail:iambsun@njupt.edu.cn;wenleizhu@nju.edu.cn;iamyangzhou@njupt.edu.cn
  • Supported by:
    the National Natural Science Foundation of China(22176086);the Natural Science Foundation of Jiangsu Province, China(BK20210189);the Natural Science Foundation of Jiangsu Province-Young Scholars Program, China(SBK2022044384);the Research Startup Fund of Nanjing University of Posts & Telecommunications, China(NY221005);the State Key Laboratory of Pollution Control and Resource Reuse of Nanjing University, China(PCRR-ZZ-202106);the Fundamental Research Funds for the Central Universities, China(021114380183);the Research Funds from Frontiers Science Center for Critical Earth Material Cycling of Nanjing University and Research Funds for Jiangsu Distinguished Professor, China(RK030STP21007)

摘要:

近年来, 随着科学研究的不断深入, 单原子催化剂由于具有高活性与高选择性等突出特点被广泛挖掘和应用. 作为连接多相与均相催化的桥梁, 单原子催化剂已经成为催化领域的重要研究对象之一, 具有广泛的工业化应用前景. 本文对单原子催化剂的发展历程、 特点及其在不同领域的应用进行了概括, 综合评述了当前CO2还原领域的技术经济分析, 并首次对单原子材料催化转化CO2进行了技术经济分析与计算. 最后, 对单原子催化剂在CO2还原领域中工业化应用的未来发展方向及亟需解决的关键科学和技术问题进行了展望, 以期推动单原子催化材料的进一步广泛应用.

关键词: 单原子, 催化, 二氧化碳还原, 技术经济分析, 工业化应用

Abstract:

In recent years, with the intensive scientific research, single-atom catalysts(SACs) have been widely explored and utilized due to their outstanding features such as high activity and high selectivity. As a bridge connec?ting heterogeneous and homogeneous catalysis, study of SACs has become one of the most important courses in the catalytic field and has broad industrial application prospects. This paper firstly gives a brief overview of the development history, characteristics and applications of SACs, and then summarizes the current techno-economic analysis in the field of CO2 reduction and presents the first techno-economic calculations for single-atom materials. Finally, the future industrial applications of SACs in CO2 reduction and the key scientific and technical issues to be solved are also discussed.

Key words: Single-atom, Catalysis, CO2 Reduction, Techno-economic analysis, Industrial application

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