Study on Three Kinds of Self-assembled Multilayer Films Prepared from Bipolar Hemicyanine Derivatives and H3PMo12O40

Chem. J. Chinese Universities

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Study on Three Kinds of Self-assembled Multilayer Films Prepared from Bipolar Hemicyanine Derivatives and H₃PMo₁₂O₄₀

WANG Yi-Bing¹, XIA Ji-Ya¹, GAO Li-Hua^1,2, WANG Ke-Zhi¹*

1. College of Chemistry, Beijing Normal University, Beijing 100875, China;
2. School of Chemical and Environment Engineering, Beijing Technology and Business University, Beijing 100037, China

Received:2006-08-26 Revised:1900-01-01 Online:2007-06-10 Published:2007-06-10
Contact: WANG Ke-Zhi

Abstract

Abstract: Three kinds of new electrostatic self-assembled multilayer films were prepared with alternating adsorption of H₃PMo₁₂O₄₀ and hemicyanine derivatives, and characterized with UV-visible absorption spectroscopy and cyclic voltammetry. The results show that these films are vertically uniform and electrochemically active with surface-controlled behavior, and the charge transfer may occur between H₃PMo₁₂O₄₀ and hemicyanine derivatives in the films. The electron transfer rates of the three films are derived to be 0.0027, 0.0019 and 0.00066 s^-1, respectively, which decrease with increasing the thickness of the hemicyanine layers in the films.

Key words: Heteropoly acid, Hemicyanine, Self-assembled film, Cyclic voltammetry, UV-visible spectroscopy

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WANG Yi-Bing¹, XIA Ji-Ya¹, GAO Li-Hua^1,2, WANG Ke-Zhi¹*. Study on Three Kinds of Self-assembled Multilayer Films Prepared from Bipolar Hemicyanine Derivatives and H₃PMo₁₂O₄₀[J]. Chem. J. Chinese Universities, doi: .

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Study on Three Kinds of Self-assembled Multilayer Films Prepared from Bipolar Hemicyanine Derivatives and H₃PMo₁₂O₄₀

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