Chem. J. Chinese Universities ›› 2023, Vol. 44 ›› Issue (6): 20220746.doi: 10.7503/cjcu20220746
• Articles: Inorganic Chemistry • Previous Articles Next Articles
LIU Jinlu, GUO Jiayu, HUA Jia, LI Guanghua(), SHI Zhan, FENG Shouhua
Received:
2022-12-06
Online:
2023-06-10
Published:
2023-01-20
Contact:
LI Guanghua
E-mail:leegh@jlu.edu.cn
Supported by:
CLC Number:
TrendMD:
LIU Jinlu, GUO Jiayu, HUA Jia, LI Guanghua, SHI Zhan, FENG Shouhua. Construction and Adsorption Properties of an Amide-based Cu-MOF[J]. Chem. J. Chinese Universities, 2023, 44(6): 20220746.
Empirical formula | C17H24CuN3O11 | Temperature/K | 293(2) |
---|---|---|---|
Formula weight | 509.93 | θ Range for data collection/(°) | 2.482—25.356 |
Crystal system | Trigonal | Limiting indice | -22≤h≤19 |
Space group | R- 3 | -21≤k≤22 | |
a/nm | 1.8947(3) | -37≤l≤45 | |
c/nm | 3.7906(8) | Reflection collected/unique/R(int) | 13454/4778/0.0778 |
Volume/nm3 | 11.785(4) | Data/restraint/parameter | 4778/30/241 |
Z | 18 | Goodness⁃of⁃fit on F2 | 0.934 |
Calculated density/(Mg·m-3) | 1.293 | R1[I>2σ(I)] | 0.0647 |
Absorption coefficient/mm-1 | 0.887 | wR2[I>2σ(I)] | 0.1688 |
F(000) | 4752 | R1(all data) | 0.1107 |
Crystal size | 0.22 mm×0.22 mm×0.18 mm | wR2(all data) | 0.1945 |
Table 1 Crystal data and structure refinement for the compound
Empirical formula | C17H24CuN3O11 | Temperature/K | 293(2) |
---|---|---|---|
Formula weight | 509.93 | θ Range for data collection/(°) | 2.482—25.356 |
Crystal system | Trigonal | Limiting indice | -22≤h≤19 |
Space group | R- 3 | -21≤k≤22 | |
a/nm | 1.8947(3) | -37≤l≤45 | |
c/nm | 3.7906(8) | Reflection collected/unique/R(int) | 13454/4778/0.0778 |
Volume/nm3 | 11.785(4) | Data/restraint/parameter | 4778/30/241 |
Z | 18 | Goodness⁃of⁃fit on F2 | 0.934 |
Calculated density/(Mg·m-3) | 1.293 | R1[I>2σ(I)] | 0.0647 |
Absorption coefficient/mm-1 | 0.887 | wR2[I>2σ(I)] | 0.1688 |
F(000) | 4752 | R1(all data) | 0.1107 |
Crystal size | 0.22 mm×0.22 mm×0.18 mm | wR2(all data) | 0.1945 |
Compound | Selectivity | Reference |
---|---|---|
ZJNU⁃55a | 13.1 | [ |
Mg⁃MOF⁃74 | 11.5 | [ |
Cu⁃PEIP | 8.9 | [ |
ZJNU⁃84 | 5.85 | [ |
[Cu(C14H7N2O5)]·5H2O·DMF | 5.52 | This work |
eea⁃MOF⁃4 | 4.3 | [ |
MOF⁃5 | 2.3 | [ |
[MIL⁃53(Al) | 2.3 | [ |
Cu3(BTC)2 | 2.3 | [ |
UMCM⁃1 | 1.8 | [ |
MOF⁃177 | 0.9 | [ |
Table 2 Comparison of the compound with other MOFs which exhibit high selectivity for CO2 over CH4 at 298 K under 101 kPa
Compound | Selectivity | Reference |
---|---|---|
ZJNU⁃55a | 13.1 | [ |
Mg⁃MOF⁃74 | 11.5 | [ |
Cu⁃PEIP | 8.9 | [ |
ZJNU⁃84 | 5.85 | [ |
[Cu(C14H7N2O5)]·5H2O·DMF | 5.52 | This work |
eea⁃MOF⁃4 | 4.3 | [ |
MOF⁃5 | 2.3 | [ |
[MIL⁃53(Al) | 2.3 | [ |
Cu3(BTC)2 | 2.3 | [ |
UMCM⁃1 | 1.8 | [ |
MOF⁃177 | 0.9 | [ |
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