Chem. J. Chinese Universities ›› 2020, Vol. 41 ›› Issue (4): 616.doi: 10.7503/cjcu20200083
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WANG Yuyao1,ZHANG Qiang1,YU Jihong1,2,*()
Received:
2020-02-19
Online:
2020-04-10
Published:
2020-03-06
Contact:
Jihong YU
E-mail:jihong@jlu.edu.cn
Supported by:
CLC Number:
TrendMD:
WANG Yuyao, ZHANG Qiang, YU Jihong. Synthesis of Hierarchical NaX Zeolite and Its CO2 Adsorption Performance †[J]. Chem. J. Chinese Universities, 2020, 41(4): 616.
Sample | x | Crystallization | Si/Al molar ratioa | Yieldb | Relative XRD crystallinityc(%) | |||
---|---|---|---|---|---|---|---|---|
Temperature/℃ | Time/h | |||||||
T1 | T2 | t1 | t2 | |||||
X-L0-60(36 h)/100(12 h) | 0 | 60 | 100 | 36 | 12 | 1.17 | 82 | 70 |
X-L1.0-60(36 h)/100(12 h) | 1.0 | 60 | 100 | 36 | 12 | 1.16 | 85 | 82 |
X-L2.0-60(36 h)/100(12 h) | 2.0 | 60 | 100 | 36 | 12 | 1.24 | 89 | 100 |
X-L0-100(24 h) | 0 | 100 | | 24 | | 1.09 | 58 | 82 |
X-L1.0-100(24 h) | 1.0 | 100 | | 24 | | 1.14 | 60 | 85 |
X-L2.0-100(24 h) | 2.0 | 100 | | 24 | | 1.21 | 64 | 97 |
Sample | x | Crystallization | Si/Al molar ratioa | Yieldb | Relative XRD crystallinityc(%) | |||
---|---|---|---|---|---|---|---|---|
Temperature/℃ | Time/h | |||||||
T1 | T2 | t1 | t2 | |||||
X-L0-60(36 h)/100(12 h) | 0 | 60 | 100 | 36 | 12 | 1.17 | 82 | 70 |
X-L1.0-60(36 h)/100(12 h) | 1.0 | 60 | 100 | 36 | 12 | 1.16 | 85 | 82 |
X-L2.0-60(36 h)/100(12 h) | 2.0 | 60 | 100 | 36 | 12 | 1.24 | 89 | 100 |
X-L0-100(24 h) | 0 | 100 | | 24 | | 1.09 | 58 | 82 |
X-L1.0-100(24 h) | 1.0 | 100 | | 24 | | 1.14 | 60 | 85 |
X-L2.0-100(24 h) | 2.0 | 100 | | 24 | | 1.21 | 64 | 97 |
Fig.1 XRD patterns of NaX samples and simulated one(A) a. Simulated; b. X-L0-60(36 h)/100(12 h); c. X-L1.0-60(36 h)/100(12 h); d. X-L2.0-60(36 h)/100(12 h). (B) a. Simulated; b. X-L0-100(24 h); c. X-L1.0-100(24 h); d. X-L2.0-100(24 h).
Fig.2 SEM images of NaX samples with or without two-step crystallization(A) X-L0-60(36 h)100(12 h); (B) X-L1.0-60(36 h)100(12 h); (C) X-L2.0-60(36 h)100(12 h); (D) X-L0-100(24 h); (E) X-L1.0-100(24 h); (F) X-L2.0-100(24 h).
Sample | (m2·g-1) | (m2·g-1) | (m2·g-1) | (cm3·g-1) | (cm3·g-1) | (cm3·g-1) |
---|---|---|---|---|---|---|
X-L0-60(36 h)/100(12 h) | 679 | 579 | 100 | 0.28 | 0.26 | 0.54 |
X-L1.0-60(36 h)/100(12 h) | 692 | 593 | 99 | 0.28 | 0.25 | 0.53 |
X-L2.0-60(36 h)/100(12 h) | 706 | 624 | 82 | 0.30 | 0.20 | 0.50 |
X-L0-100(24 h) | 652 | 573 | 79 | 0.27 | 0.10 | 0.37 |
Sample | (m2·g-1) | (m2·g-1) | (m2·g-1) | (cm3·g-1) | (cm3·g-1) | (cm3·g-1) |
---|---|---|---|---|---|---|
X-L0-60(36 h)/100(12 h) | 679 | 579 | 100 | 0.28 | 0.26 | 0.54 |
X-L1.0-60(36 h)/100(12 h) | 692 | 593 | 99 | 0.28 | 0.25 | 0.53 |
X-L2.0-60(36 h)/100(12 h) | 706 | 624 | 82 | 0.30 | 0.20 | 0.50 |
X-L0-100(24 h) | 652 | 573 | 79 | 0.27 | 0.10 | 0.37 |
Fig.4 XRD patterns of samples with different crystallization timea. X-L2.0-60(36 h); b. X-L2.0-60(36 h)/100(1 h); c. X-L2.0-60(36 h)/100(2 h); d. X-L2.0-60(36 h)/100(4 h); e. X-L2.0-60(36 h)/100(12 h).
Fig.5 TEM images of crystal evolution under 100 ℃ for samples X-L2.0-60(36 h)/100(1 h)(A), X-L2.0-60(36 h)/100(2 h)(B) and X-L2.0-60(36 h)/100(12 h)(C)
Sample | Adsorption quantitity | |
---|---|---|
273 K | 298 K | |
X-L1.0-60(36 h)/100(12 h) | 154.2 | 140.6 |
X-L2.0-60(36 h)/100(12 h) | 151.9 | 142.4 |
X-L0-100(24 h) | 147.6 | 129.2 |
Sample | Adsorption quantitity | |
---|---|---|
273 K | 298 K | |
X-L1.0-60(36 h)/100(12 h) | 154.2 | 140.6 |
X-L2.0-60(36 h)/100(12 h) | 151.9 | 142.4 |
X-L0-100(24 h) | 147.6 | 129.2 |
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