高等学校化学学报 ›› 2019, Vol. 40 ›› Issue (9): 1988.doi: 10.7503/cjcu20190030
收稿日期:
2019-01-14
出版日期:
2019-09-10
发布日期:
2019-09-09
通讯作者:
马永钧
E-mail:mayj@nwnu.edu.cn
基金资助:
LIU Fen,ZHOU Min,WANG Suxia,WANG Rong,YANG Ning,MA Yongjun()
Received:
2019-01-14
Online:
2019-09-10
Published:
2019-09-09
Contact:
MA Yongjun
E-mail:mayj@nwnu.edu.cn
Supported by:
中图分类号:
TrendMD:
刘芬, 周敏, 王苏霞, 王荣, 杨宁, 马永钧. 用化学需氧量指数法研究亚甲基蓝的可见光光电催化脱色反应机理. 高等学校化学学报, 2019, 40(9): 1988.
LIU Fen, ZHOU Min, WANG Suxia, WANG Rong, YANG Ning, MA Yongjun. Study on Photoelectrocatalytic Decolorization Mechanism of Methylene Blue Under the Visible-light Irradiation by Measuring Chemical Oxygen Demand Index†. Chem. J. Chinese Universities, 2019, 40(9): 1988.
Fig.1 SEM images of modified photoelectrodes CuInSe2/GC(A), CuInSe2/Ag3PO4@AgIO4/GC(B) and TEM images of CuInSe2/Ag3PO4@AgIO4 granular catalyst material(C, D)
Fig.3 Effect of pH value of supporting electrolyte on the decoloration efficiency of MB dye in the visible-light photoelectrocatalytic reaction H2O2 initial concentation: 0.42 mol/L; reaction temperature: 50 ℃; irradiation time: 45 min.
Fig.4 Influence of applied bias voltage on the degradation efficiency of MB dye in the visible-light photoelectrocatalytic reaction(A) and the voltammogram of MB testing solution using linear sweep voltammetry(LSV) under the visible-light irradiation condition(B)
pH | 2.7 | 3.7 |
---|---|---|
Decoloration rate, D(%) | 86.0 | 54.0 |
η*(%) | 45.0 | 20.8 |
η**(%) | 16.3 | 6.8 |
MB Mineralization rate, Ma (%) | 10.1 | 3.7 |
D/M ratio | 8.5 | 14.6 |
Table 1 Comparison between the decoloration rate and COD removal rate of MB dye at the different acidity conditions of MB+H2O2 system
pH | 2.7 | 3.7 |
---|---|---|
Decoloration rate, D(%) | 86.0 | 54.0 |
η*(%) | 45.0 | 20.8 |
η**(%) | 16.3 | 6.8 |
MB Mineralization rate, Ma (%) | 10.1 | 3.7 |
D/M ratio | 8.5 | 14.6 |
Fig.5 Influence of irradiation time on ultraviolet-visible absorption spectra(A) and the degradation efficiency of MB dye(B) Curves a—c represen the decoloration rate(D), COD removal rate of the supernatant fraction(η*) and total COD removal rate(η**), respectively.
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