Laser-mediated Enrichment Based Surface Enhanced Raman Analysis

doi:10.7503/cjcu20210153

Abstract

Abstract:

Surface enhanced Raman scattering（SERS） technique has extensive application prospects in biochemical analysis and environmental monitoring field owing to its high sensitivity， low background inter- ference， superior anti-photobleaching and anti-photocarbonization capabilities， as well as ability to reflect the inherent molecular fingerprint information of the analyte. Non-target analytes are competitively adsorbed on the surface of the SERS substrate， making the analysis of trace analytes in complex systems extremely challenging. Based on the self-assemble of the graphene-isolated Au nanocrystal（GIAN） with excellent SERS performance at H₂O-Organic phase interface， the large partition coefficient of the analyte in organic phase， and GIAN can combine with the analyte viaπ-π interaction， a laser-mediated highly-efficient analyte enrichment strategy is proposed and trace SERS analysis of 9，10-bis（phenylethynyl）anthracene（BPEA） molecules is eventually realized in this work. The proposed novel analyte enrichment strategy avoids the signal fluctuation caused by the “coffee ring effect” to a certain extent and is expected to provide a reliable platform for SERS analysis of trace analytes in complex systems.

Key words: Laser-mediated enrichment, Surface enhanced Raman scattering, Two-phase interface, Graphene-isolated Au nanocrystal, Self-assembly

CLC Number:

O657.37

TrendMD:

TANG Wentao, LI Shengkai, WANG Shen, CHEN Long, CHEN Zhuo. Laser-mediated Enrichment Based Surface Enhanced Raman Analysis[J]. Chem. J. Chinese Universities, 2021, 42(10): 3054.

Figures/Tables 9

References 29

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