高等学校化学学报 ›› 2023, Vol. 44 ›› Issue (1): 20220586.doi: 10.7503/cjcu20220586
收稿日期:
2022-09-02
出版日期:
2023-01-10
发布日期:
2022-10-14
通讯作者:
陈晨
E-mail:cchen@mail.tsinghua.edu.cn
基金资助:
Received:
2022-09-02
Online:
2023-01-10
Published:
2022-10-14
Contact:
CHEN Chen
E-mail:cchen@mail.tsinghua.edu.cn
Supported by:
摘要:
由超薄边框相互连接形成的贵金属纳米框架以负载量低、 活性高等优势在多相催化领域受到了广泛关注. 纳米框架独特的三维开放可及性结构不仅能够在边缘和顶点处暴露出更多的活性位点, 提高贵金属活性位点利用率, 还可以将反应底物限制在纳米范围内, 增加底物分子碰撞的几率. 本文综合评述了贵金属纳米框架材料的合成策略, 总结了近年来贵金属纳米框架催化剂在电催化领域的研究进展, 并对其未来发展方向和面临的挑战进行了展望.
中图分类号:
TrendMD:
匡华艺, 陈晨. 贵金属纳米框架设计合成及电催化性能的研究进展. 高等学校化学学报, 2023, 44(1): 20220586.
KUANG Huayi, CHEN Chen. Synthesis Methods and Electrocatalytic Performance of Noble-metal Nanoframes Catalysts. Chem. J. Chinese Universities, 2023, 44(1): 20220586.
Fig.2 Schematic illustrations and corresponding transmission electron microscope(TEM) images of the samples obtained at four representative stages during the evolution process from polyhedra to nanoframes[10](A) Initial solid PtNi3 polyhedra; (B) PtNi intermediates; (C) final hollow Pt3Ni nanoframes; (D) annealed Pt3Ni nanoframes with Pt(111)-skin-like surfaces dispersed on high-surface area carbon.Copyright 2014, American Association for the Advancement of Science.
Fig.3 Elemental mapping, HAADF⁃STEM images, and EDX line scan profiles of Pt3Ni tetrahexahedral nanoframes(A—C), yielded via CO⁃annealing at 170 °C for 45 min. HAADF⁃STEM image on a selected nanoframes in the zone axis of [001], showing its Pt⁃rich hollow structure and Ni removal(D)[16]Copyright 2017, American Chemical Society.
Fig.4 Schematic illustration of the growth mechanism of Au nanoframes[17]Ag+ and Br- ions show a synergistic function to obtain Au nanoframes.Copyright 2020, American Chemical Society.
Fig.5 Schematic illustration showing the two steps involved in the synthesis of Ru NFs(A) and schematic illustrations summarizing the different pathways and the corresponding morphologies expected for the overgrowth of Ru on a Pd truncated octahedral seed under three different conditions(B)[22](A) (1) Selective nucleation and growth of Ru on the corners and edges of Pd truncated octahedra, yielding Pd-Ru core-frame octahedra; (2) formation of Ru octahedral NFs by etching away the Pd cores. Copyright 2016, American Chemical Society.
Fig.7 Core⁃shell Cu⁃Pt polyhedra observed at different stages during structure transformation[25]TEM images(A1—D1), HRTEM images(A2—D2), and corresponding schematic illustrations(A3—D3) to show the core-shell Cu-Pt polyhedra aging in toluene for 0 d(A series), 14 d(B series), 21 d(C series), and 28 d(D series), respectively.
Fig.8 Morphological evolution of Ag nanoparticles to Au3Ag nanoframes[28]SEM(A) and TEM(B) overview of Au3Ag nanoframes showing high structural uniformity. The schematic diagram, SEM, TEM, and EDX mapping images of Ag NPs(C) collected at the 36th min before HAuCl4 addition, AuAg12 NPs collected at the 38th min after HAuCl4 addition(D), Au2Ag NCs collected at the 42th min(E), and Au3Ag NFs collected at the 46th min(F).Copyright 2019, The Author(s).
Fig.9 TEM images of different shapes of triangular nanoframes(A—D) and the schematic illustration of their formation(E)(scale bar: 50 nm)[31]Copyright 2017, Wiley-VCH VERLAG GMBH & Co. KGAA.
Fig.10 Schematic illustration of the synthetic strategy for the atomically ordered intermetallic PtCu nanoframes[43]Copyright 2020, American Chemical Society.
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