Construction of High Efficiency Uric Acid Sensor Based on the co-Crystal Enhanced Electrochemiluminescence from 9,10-Diphenylanthracene-perylene Microcrystals

doi:10.7503/cjcu20200294

Abstract

Abstract:

A new luminophore with co-crystal enhanced electrochemiluminescence(ECL) was obtained by the surfactant assisted self-assembly of the non-coplanar molecule 9,10-diphenylanthracene(DPA) and planar molecule perylene(Pe). The introduction of DPA in the co-crystals can not only reduce the aggregation-caused quenching(ACQ) effect of perylene, making the ECL emission of Pe molecule from the dimer or multimer excited state(¹Pe^2*) to the monomer excited state(¹Pe^*), but also plays a role as a donor molecule, providing effective energy transfer to the acceptor molecule of Pe, which further enhances the ECL response. The electrochemical sensor for uric acid based on DPA-Pe microcrystals has an extremely wide linear of 0.01 μmol/L—5.0 mmol/L and a detection limit of 4.0 nmol/L. In addition, the sensor has a nice stability and selectivity for uric acid detection.

Key words: co-Crystal enhanced electrochemiluminescence, 9,10-Diphenylanthracene, Perylene, Uric acid, Sensor

CLC Number:

O657

TrendMD:

LIAO Ni, ZHANG Jieyuan, HUANG Ziyang, ZHAO Yanxi, CHAI Yaqin, YUAN Ruo, ZHUO Ying. Construction of High Efficiency Uric Acid Sensor Based on the co-Crystal Enhanced Electrochemiluminescence from 9,10-Diphenylanthracene-perylene Microcrystals[J]. Chem. J. Chinese Universities, 2020, 41(9): 1989.

Figures/Tables 6

References 19

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