doi:10.7503/cjcu20170660

Figures/Tables 8

Scheme 1 Synthesis process of Pyrene-1

Table 1 Preparation conditions of pyrene-doped silica fluorescent nanoparticles*

Sample	P₁	P_0.5	P_0.25	P_0.1	P_0.05	P_0.01
m(Pyrene-1)/mg	3.93	1.97	0.98	0.39	0.20	0.04
V(TEOS)/μL	180	180	180	180	180	180
n(Pyrene-1)∶n(TEOS)	1∶100	0.5∶100	0.25∶100	0.1∶100	0.05∶100	0.01∶100

Scheme 2 Schematic illustration of Pyrene-doped silica nanoparticles

Fig.1 Diameter distribution of pyrene-doped silica fluorescent nanoparticles Note: (A) P1; (B) P0.5; (C) P0.25; (D) P0.1; (E) P0.05; (F) P0.01. Insets: TEM images of corresponding pyrene-doped silica fluorescent nanoparticles.

Fig.2 DLS results of pyrene-doped silica fluorescent nanoparticle Note:(A) P1; (B) P0.5; (C) P0.25; (D) P0.1; (E) P0.05; (F) P0.01.

Fig.3 Absorption(A, C) and emission(B, D) spectra of pyrene-doped silica fluorescent nanoparticles(A, B) and pyrene-1 in chloroform(C, D) Note:(A) c=1 μmol/L, λex=345 nm; (B) c=10 μmol/L, λex=345 nm.

Fig.4 Histograms of fluorescence quantum yields(A) and lifetimes(B) of pyrene-1 in different media

Fig.5 Fluorescence patterning of TIPC written by P1 and P0.1 under the UV lamp λex=254 nm.

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