Construction of Double S-scheme YVO4/TiO2/BiVO4 Heterojunction and Its Photocatalytic CO2 Reduction Performance

doi:10.7503/cjcu20240298

Abstract

Abstract:

The double S-scheme heterojunction of YVO₄/TiO₂/BiVO₄ compoite fibers material was prepared by one-step hydrothermal method using TiO₂ electrospun nanofibers as substrate. The structures of the composite catalyst were characterized by X-ray diffraction， scanning electron microscopy， transmission electron microscopy， X-ray photoelectron spectroscopy， ultraviolet visible diffuse reffectance spectroscopy and photoluminescence. The performance of photocatalytic CO₂ reduction over the composite catalyst under simulated sunlight was studied. The results show that photocatalytic activity of YVO₄/TiO₂/BiVO₄ composite fibers was investigated via production of methanogenesis from photocatalytic reduction of CO₂. The CO₂ reduction capability of composite fibers was better compared to that of monomer materials. The photocatalytic production rate of CH₄ and CH₃OH of YVO₄/TiO₂/BiVO₄ were 13.88 and 3.46 μmol·g^‒1·h^‒1， respectively. The increased photocatalytic activity of YVO₄/TiO₂/BiVO₄ is attributed to the formation of heterojunctions between YVO_4，BiVO₄ and TiO₂ as well as the S‐scheme charge transfer mode of the photogenerated carriers， both of which are conducive to separation efficiency of photo‐generated carriers and photocatalytic CO₂reduction activity.

Key words: S-scheme heterojunction, Composite fiber, Electrospinning, Photocatalytic CO₂ reduction

CLC Number:

O643

TrendMD:

CAO Tieping, LI Yuejun, SUN Dawei. Construction of Double S-scheme YVO₄/TiO₂/BiVO₄ Heterojunction and Its Photocatalytic CO₂ Reduction Performance[J]. Chem. J. Chinese Universities, 2024, 45(12): 20240298.

Figures/Tables 10

References 25

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Construction of Double S-scheme YVO₄/TiO₂/BiVO₄ Heterojunction and Its Photocatalytic CO₂ Reduction Performance

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