Chem. J. Chinese Universities ›› 2020, Vol. 41 ›› Issue (4): 604.doi: 10.7503/cjcu20190641
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LI Zhenhua1,2,SHI Run1,ZHAO Jiaqi1,ZHANG Tierui1,2,*()
Received:
2019-12-09
Online:
2020-04-10
Published:
2020-02-24
Contact:
Tierui ZHANG
E-mail:tierui@mail.ipc.ac.cn
Supported by:
CLC Number:
TrendMD:
LI Zhenhua, SHI Run, ZHAO Jiaqi, ZHANG Tierui. Research Progress of Photo-driven C1 Conversion to Value-added Chemicals †[J]. Chem. J. Chinese Universities, 2020, 41(4): 604.
Fig.1 Schematic showing the reaction process FTS over Ru/graphene under light irradiation(A) and selectivities of photocatalytic FTS hydrocarbons with or without irradiation at different temperatures(B)[46]Copyright 2015, American Chemical Society.
Fig.2 Potential-energy profile of the most possible reaction paths for syngas conversion on Ni(111) and 4O/Ni(111)(A)[47], fabrication of Co-x catalysts and their light-driven FTS performance(B)[48], the potential energy profile of CO dissociation on Co3O4(220), Co(111)/Co3O4(220), and Co(111), CH2 coupling and C2H4 hydrogenation on Co(111)/Co3O4(220) and Co(111)(C)[48], reductive transformation of ZnFeAl-LDH nanosheets to Fe-x catalysts and their photocatalytic behavior in FTS(D)[49] and energy profiles for CO2 formation, C2H4 adsorption and hydrogenation(E)[49](A) Copyright 2016, Wiley-VCH; (B, C) Copyright 2018, Wiley-VCH; (D, E) Copyright 2018, Wiley-VCH.
Fig.3 Two possible mechanisms to rationalize the differences in the UV-Vis or visible light photocatalytic activity of Au/TiO2(A)[52], temporal profile of CO consumption(a), CO2 evolution(b) and H2 evolution(c) over a Au/TiO2(1%) catalyst under solar light irradiation(B)[52], H2 evolution rates and CO conversion of CuOx/Al2O3-19, CuOx/Al2O3-2, Pt/Al2O3-2 and Au/Al2O3-2 catalysts(C)[53] and cycling measurements of WGS reaction under photothermal condition over CuOx/Al2O3 catalyst(D)[53](A, B) Copyright 2013, Royal Society of Chemistry; (C, D) Copyright 2019, Wiley-VCH.
Fig.4 Schematic of CF-Cu2O growth process from the Cu foam precursor(A) and long-term stability of CF-Cu2O in an LED flow reactor(B)[57]Copyright 2019, Nature Publishing Group.
Fig.5 Reaction mechanism for CO and CH4 evolution on a rhodium nanocube(A)[58], schematic presence of the formation of ultrathin LDH structure with abundant surface hydroxyl groups(B)[60] and photothermal conversion of CO2 and cumulative yield of CH4 over Ru loaded catalysts under different flow rates(F. R. ) of CO2 and H2 mixture(C) [60](C) S1: Ru@FL-LDHs; S2: Ru@LDHs; S3: Ru@SiO2. (A) Copyright 2017,Nature Publishing Group; (B, C) Copyright 2016, Wiley-VCH.
Fig.6 Illustration of the different CoFe-x catalysts formed by hydrogen reduction of CoFeAl-LDH nanosheets at different temperatures and their catalytic activities for CO2 hydrogenation(A), time course of CO2 conversion and product selectivities for CO2 hydrogenation over CoFe-650 under UV-Vis irradiation(B) and the hydrocarbon product distribution obtained over CoFe-650 under UV-Vis irradiation for 2 h(C)[61]Copyright 2018, Wiley-VCH.
Fig.7 Schematic of energy transfer from photoexcited hot carriers to adsorbate states and proposed mechanism for SRM reaction on Rh/TiO2 under visible light illumination(A)[65], a schematic illustration of the solar-light-driven thermocatalytic(B) and the catalytic activity of SCM-Ni/SiO2 for CRM versus reaction time under the focused full-solar-spectrum irradiation from the Xe lamp(C)[66](A) Copyright 2018, American Chemical Society; (B, C) Copyright 2018, Wiley-VCH.
Fig.8 Synthesis and methanol photocatalytic application of single-layer MoS2 nanosheets(A), effects of surfactant, methanol, and photocatalysts on MTH efficiency between three different samples while keeping all other experimental conditions the same(B) and DFT calculations(C)[68](B) Sample 1: 10 mL(ca. 8.2 × 103 mg) pure surfactant; sample 2: 5 mL surfactant and 5 mL methanol; sample 3: 2 mg MoS2 in 10 mL methanol. Copyright 2019, Wiley-VCH.
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