Physical Absorption of CO2 Using Polyvinylidene Fluoride Membrane Contactor at High Pressure and Mathematical Simulation

doi:10.7503/cjcu20120881

Abstract

Abstract:

The removal of CO₂ from natural gas using polyvinylidene fluoride(PVDF) hollow fiber membrane contactor was studied at high pressure. The distilled water was used as absorbent. The effects of operating pressure, inlet gas flow rate and liquid flow rate on removal efficiency of CO₂ were investigated. Based on the physical mass transfer process, the mass transfer equation of gas phase, membrane phase and liquid phase were established. The outlet CO₂ content could be predicted using Multiphysics(COMSOL) combined with 2-D mathematical model and corresponding boundary conditions. The results showed that the removal efficiency of CO₂ was affected significantly by the partial wetting of membrane. The predicted results were in good agreement with the experimental data if the wetting ratio of membrane was considered in the mathematical model.

Key words: Hollow fiber membrane contactor, High pressure, Physical absorption, CO₂, Mathematical model

CLC Number:

O647.32

TrendMD:

HUA Cong-Gui, KANG Guo-Dong, JIA Jing-Xuan, LI Meng, CAO Yi-Ming, YUAN Quan. Physical Absorption of CO₂ Using Polyvinylidene Fluoride Membrane Contactor at High Pressure and Mathematical Simulation[J]. Chem. J. Chinese Universities, 2013, 34(4): 906.

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Physical Absorption of CO₂ Using Polyvinylidene Fluoride Membrane Contactor at High Pressure and Mathematical Simulation

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