Electrogenerated Chemiluminescence Biosensor Based on Ru(bpy)32+ Doped Mesoporous Silica Nanoparticles

doi:10.3969/j.issn.0251-0790.2012.06.008

Abstract

Abstract: A novel electrogenerated chemiluminescence(ECL) sensor based on Ru(bpy)₃²⁺-doped MCM-41 mesoporous silica nanoparticles(MSN) was developed. The Ru(bpy)₃²⁺ was first loaded into the sulfhydryl modified MSN through the electrostatic absorption. Then the Ru(bpy)₃²⁺-doped MSN was immobilized onto the surface of Au electrode by Au-S interaction. The properties of electrochemistry and electrogenerated chemiluminescence(ECL) were also investigated. The amino structure of melamine is similar to tripropylamine, so we attempted to branch out the application of MCM-41 into the detection of melamine, the ECL sensor provided a new assay for the detection of melamine. Furthermore, the research provided a new approach for the immobilization of Ru(bpy)₃²⁺ onto the electrode surface.

Key words: Mesoporous silica nanoparticles, Electrogenerated chemiluminescence, Ru(bpy)₃²⁺, Melamine

CLC Number:

O657.1

TrendMD:

WANG Yong-Hong, HE Xiao-Xiao, WANG Ke-Min, SU Jing, CHEN Zhi-Feng, YAN Gen-Ping. Electrogenerated Chemiluminescence Biosensor Based on Ru(bpy)₃²⁺ Doped Mesoporous Silica Nanoparticles[J]. Chem. J. Chinese Universities, 2012, 33(06): 1162.

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Electrogenerated Chemiluminescence Biosensor Based on Ru(bpy)₃²⁺ Doped Mesoporous Silica Nanoparticles

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