Chem. J. Chinese Universities ›› 2014, Vol. 35 ›› Issue (1): 92.doi: 10.7503/cjcu20130808
• Physical Chemistry • Previous Articles Next Articles
HE Zhanfeng1,2, WANG Dan1,2, LIU Tao1,2, WANG Huanyi1,2, JIANG Yi1,*()
Received:
2013-08-20
Online:
2014-01-10
Published:
2013-12-04
Contact:
JIANG Yi
E-mail:yjiang@cioc.ac.cn
Supported by:
CLC Number:
TrendMD:
HE Zhanfeng, WANG Dan, LIU Tao, WANG Huanyi, JIANG Yi. Nb-modified Pd/Al2O3 Catalysts for Benzene Catalytic Combustion†[J]. Chem. J. Chinese Universities, 2014, 35(1): 92.
Sample | Surface area/(m2·g-1) | Pore volume/(cm3·g-1) | Sample | Surface area/(m2·g-1) | Pore volume/(cm3·g-1) |
---|---|---|---|---|---|
Al2O3 | 184 | 0.34 | 5%Nb/Al2O3 | 176 | 0.32 |
1%Pd/Al2O3 | 179 | 0.33 | 1%Pd-5%Nb/Al2O3 | 172 | 0.31 |
2%Pd/Al2O3 | 174 | 0.32 |
Table 1 Textural properties of different catalysts and supports
Sample | Surface area/(m2·g-1) | Pore volume/(cm3·g-1) | Sample | Surface area/(m2·g-1) | Pore volume/(cm3·g-1) |
---|---|---|---|---|---|
Al2O3 | 184 | 0.34 | 5%Nb/Al2O3 | 176 | 0.32 |
1%Pd/Al2O3 | 179 | 0.33 | 1%Pd-5%Nb/Al2O3 | 172 | 0.31 |
2%Pd/Al2O3 | 174 | 0.32 |
Catalyst | Elemental content(%) | Eb/eV | ||||||||
---|---|---|---|---|---|---|---|---|---|---|
Pd | Nb | Al | O | P | P | N | Al2p | O1s | ||
5%Nb/Al2O3 | 1.3 | 36.0 | 63.0 | 207.2 | 74.4 | 531.4 | ||||
1%Pd/Al2O3 | 0.30 | 36.3 | 63.4 | 336.5 | 74.4 | 531.5 | ||||
1%Pd-5%Nb/Al2O3 | 0.40 | 1.4 | 32.2 | 66.0 | 335.7 | 337.1 | 207.5 | 74.4 | 531.8 |
Table 2 Elemental content and binding energy on the catalyst surface
Catalyst | Elemental content(%) | Eb/eV | ||||||||
---|---|---|---|---|---|---|---|---|---|---|
Pd | Nb | Al | O | P | P | N | Al2p | O1s | ||
5%Nb/Al2O3 | 1.3 | 36.0 | 63.0 | 207.2 | 74.4 | 531.4 | ||||
1%Pd/Al2O3 | 0.30 | 36.3 | 63.4 | 336.5 | 74.4 | 531.5 | ||||
1%Pd-5%Nb/Al2O3 | 0.40 | 1.4 | 32.2 | 66.0 | 335.7 | 337.1 | 207.5 | 74.4 | 531.8 |
[1] | Garin F., Catal Today, 2004, 89(3), 255—268 |
[2] | Prasad R., Kennedy L. A., Ruckenstein E., Catal. Rev., 1984, 26(1), 1—58 |
[3] | Ye Q., Huo F. F., Wang H. P., Wang J., Wang D., Chem. J. Chinese Universities, 2013, 34(5), 1187—1194 |
(叶青, 霍飞飞, 王海平, 王娟, 王道.高等学校化学学报, 2013,34(5), 1187—1194) | |
[4] | Andrzej C., Jacob A. M., Catal. Rev., 1994, 36(2), 179—270 |
[5] | Yao Y. L., Shi Z. H., Song W. C., Yuan S. H., Gong M. C., Chen Y. Q., Chin. J. Catal., 2008, 29(4), 316—318 |
(姚艳玲, 史忠华, 宋为聪, 袁书华, 龚茂初, 陈耀强.催化学报, 2008,29(4), 316—318) | |
[6] | Liu Z. M., Wang J. L., Zhong J. B., Chen Y. Q., Yan S. H., Gong M. C., J. Hazard. Mater., 2007, 149(3), 742—746 |
[7] | Ferreira R. S. G., Oliveira P. G. P., Noronha F. B., Appl. Catal. B, 2004, 50(4), 243—249 |
[8] | Huang S. Y., Zhang C. B., He H., Catal. Today, 2008, 139(1/2), 15—23 |
[9] | Wang J. L., Liu Z. M., Cong H. Y., Chen Y. D., Gong M. C., Chen Y. Q., Chem. Res. Chinese Universities, 2009, 25(1), 81—85 |
[10] | Qiao B. T., Wang A. Q., Yang X. F., Lawrence F. A., Jiang Z., Cui Y. T., Liu J. Y., Li J., Zhang T., Nat. Chem., 2011, 3, 634—641 |
[11] | Zhang C. B., Liu F. D., Zhai Y. P., Ariga H., Yi N., Liu Y. C., Asakura K. Y., Flytzani-Stephanopoulos M., He H., Angew. Chem. Int. Ed., 2012, 51(38), 9628—9632 |
[12] | Qi C. Z., Zuo S. F., Catal. Common., 2011, 15(1), 74—77 |
[13] | Padilla J. M., Angel G. D., Navarrete J., Catal. Today, 2008, 133—135, 541—547 |
[14] | Konopny L. K., Juan A., Damiania D. E., Appl. Catal. B, 1998, 15(1/2), 115—127 |
[15] | Kinnunen N. M., Suvanto M., Moreno M. A., Savimäki A., Kallinen K., Kinnunen T. J. J., Pakkanen T. A., Appl. Catal. A, 2009, 370(1/2), 78—87 |
[16] | Okumura K., Kobayashi T., Tanaka H., Niwa M., Appl. Catal. B, 2003, 44(4), 325—331 |
[17] | Yazawa Y., Yoshida H., Komai S., Hattori T., Appl. Catal. A, 2002, 233(1/2), 113—124 |
[18] | Ziolek M., Catal. Today, 2003, 78(1—4), 47—64 |
[19] | Lieske H., Völter J., J. Phys. Chem. C, 1985, 85(10), 1841—1842 |
[20] | Jin R. B., Liu Y., Wu Z. B., Wang H. Q., Gu T. T., Chemosphere, 2010, 78(9), 1160—1166 |
[21] | Mhamdi M., Khaddar-Zine S., Ghorbel A., Appl. Catal. A, 2009, 357(1/2), 42—50 |
[22] | Yazawa Y., Yoshida H., Takagi N., Kagi N., Komai S., Satsuma A., Murakami Y., Hattori T., Stud. Surf. Sci.Catal., 2000, 130,2189—2194 |
[23] | Kili K., Hilaire L., Normand F. L., Phys. Chem. Chem. Phys., 1999, 1(7), 1623—1631 |
[24] | Venezia A. M., Rossi A., Duca D., Martorana A., Deganello G., Appl. Catal. A, 1995, 125(1), 113—128 |
[25] | Gao D. N., Zhang C. X., Wang S., Yuan Z. S., Wang S. D., Catal. Commun., 2008, 9(15), 2583—2587 |
[26] | Yazawa Y., Yoshida H., Takagi N., Kagi N., Komai S., Satsuma A., Murakami Y., Hattori T., J. Catal., 1999, 187(1), 15—23 |
[1] | LIU Suyu, DING Fei, LI Qian, FAN Chunhai, FENG Jing. Azobenzene-integrated DNA Nanomachine [J]. Chem. J. Chinese Universities, 2022, 43(8): 20220122. |
[2] | GAO Jian, FENG Yiyu, FANG Wenyu, WANG Hui, GE Jing, FENG Wei. Alkane Grafted Phase Change Azobenzene Materials Based on Low Temperature Heat Release [J]. Chem. J. Chinese Universities, 2022, 43(8): 20220146. |
[3] | WANG Gaobo, MA Jing. Binding Selectivity Between Diazobenzene and Different Nucleophilic Reagents: Covalent and Noncovalent Interactions [J]. Chem. J. Chinese Universities, 2021, 42(7): 2238. |
[4] | LI Xinyu, LI Zhiwei, ZHANG Xingyuan. Construction of Room Temperature Phosphorescence System of Thioflavin-based Polylactide/Benzenesulfonic Acid [J]. Chem. J. Chinese Universities, 2021, 42(6): 1987. |
[5] | WU Shuaini, ZHU Pengfei, SHI Huaiqi, LI Na, HU Zhaoxia, CHEN Shouwen. Preparation of CoCrx/SAPO-34 Catalyst and Its Catalytic Combustion Performance for 1,2-Dichloroethane [J]. Chem. J. Chinese Universities, 2021, 42(12): 3731. |
[6] | ZHU Min, ZHANG Xiao, YOU Shuli. Visible-light-promoted Dearomatization of Benzene and Derivatives† [J]. Chem. J. Chinese Universities, 2020, 41(7): 1407. |
[7] | LI Shanshan, ZHAO Wenjuan, LI Hui, FANG Qianrong. A Photoresponsive Azobenzene-functionalized Covalent Organic Framework [J]. Chem. J. Chinese Universities, 2020, 41(6): 1384. |
[8] | BAI Ruonan, LI Qing, QIAO Shanlin, ZHANG Chunhuan, ZHAO Yongsheng. Controlled Preparation and Optical Waveguide Property of 1,4-Dicarbazolidinylbenzene Microwires [J]. Chem. J. Chinese Universities, 2020, 41(5): 967. |
[9] | DONG Xinrui, XIA Zhe, WANG Zhenxue, BIAN Qiang, LI Huabin. Design, Synthesis and Biological Activity of Pyrazole-4-carboxamides Compounds Containing 1,2,4,5-Tetrasubstituted Phenyl [J]. Chem. J. Chinese Universities, 2020, 41(12): 2759. |
[10] | ZHANG Hui, ZHANG Chenjie, XU Minmin, YUAN Yaxian, YAO Jianlin. Investigation on the Reaction of o-Aminothiophenol and 2-Iodobenzoyl Chloride Monitored by SERS-HPLC Technique [J]. Chem. J. Chinese Universities, 2020, 41(11): 2496. |
[11] | WANG Yue, GUO Xiaohong, ZHOU Guangdong, CHENG Tiexin. Effect of Alkyl Benzene Sulfonate Surfactant on Morphology and Structure of Calcium Silicate Hydrate † [J]. Chem. J. Chinese Universities, 2019, 40(9): 1795. |
[12] | HU Xueyi, CHEN Miaomiao, FANG Yun, FENG Ruiqin, HAN Huihui. Investigation on Pseudo-polyanions of Cationic Cellulose-Sodium Dodecylbenzenesulfonate† [J]. Chem. J. Chinese Universities, 2019, 40(7): 1464. |
[13] | BIAN Kai, HOU Zhanggui, DUAN Xinrui, LI Xiaoguo, CHANG Yang, CAO Hui, ZHANG Anfeng, GUO Xinwen. Synthesis and Catalytic Performance of 2D HZSM-5 Nano-sheet for Ethylbenzene Production from Benzene with Dilute Ethylene [J]. Chem. J. Chinese Universities, 2019, 40(4): 784. |
[14] | ZHAO Ruiyang,YU Chunyan,HAN Jishu,FU Yunlei,LI Ming,HU Dehua,LIU Fusheng. Preparation of Photo-responsive Film by Electrochemical Deposition Method and the Application in Optical Information Storage† [J]. Chem. J. Chinese Universities, 2019, 40(2): 358. |
[15] | Siqi SUN,Ying WANG,Chuanyin SUN,Runwei WANG,Zhendong ZHANG,Zongtao ZHANG,Shilun QIU. Preparation and Catalytic Performance of Bowl-shaped Amphiphilic ZSM-5 Zeolites Supported Gold Nanoparticles † [J]. Chem. J. Chinese Universities, 2019, 40(12): 2436. |
Viewed | ||||||
Full text |
|
|||||
Abstract |
|
|||||