Synthesis and Fluorescence Behavior of Acceptor-donor-acceptor Type Bismaleimides

Abstract

Abstract: Bismaleimides bearing electron-donating chromophore moieties, A₍₌₎-D_(*)-A₍₌₎ type monomers, i.e. N,N-bis(4-maleimidophenyl)methylamine (BMIPMA), N,N-bis(4-maleimidophenyl)aniline(BMIPA) and 2,5-bis(4-maleimido phenyl)-1,3,4-oxadiazole(BMIPODA) as well as their corresponding saturated model compounds, i.e. N,N-bis(4-succinimidophenyl)methylamine( BSIPMA), N,N-bis(4-succinimidophenyl)aniline(BSIPA) and 2,5-bis(4-succimidophenyl)-1,3,4-oxadiazole (BSIPODA) were synthesized. It was found that the fluorescence quantum yields of A₍₌₎-D_(*)-A₍₌₎ monomers were always dramatically lower than those of their corresponding saturated model compounds. These A₍₌₎-D_(*)-A₍₌₎ bismaleimides possess a strong SSQE, which is attributed to an intramolecular charge transfer interaction.

Key words: Fluorescence, Structural self-quenching effect(SSQE), Bismaleimides, Charge transfer complex

CLC Number:

O631.1

TrendMD:

ZHANG Xin, JIN Ying-Hua, DU Fu-Sheng, LI Zi-Chen, LI Fu-Mian . Synthesis and Fluorescence Behavior of Acceptor-donor-acceptor Type Bismaleimides[J]. Chem. J. Chinese Universities, 2003, 24(2): 365.

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Synthesis and Fluorescence Behavior of Acceptor-donor-acceptor Type Bismaleimides

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