Chem. J. Chinese Universities ›› 2021, Vol. 42 ›› Issue (2): 556.doi: 10.7503/cjcu20200565

• Review • Previous Articles     Next Articles

Synthesis and Electrocatalytic Application of Two-dimensional Metal-organic Frameworks

JIANG Qinyuan, ZHOU Chenhui, MENG Haibing, HAN Ying, ZHANG Rufan()   

  1. Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology,Engineering Research Center of Clean Energy Chemical Technology,Ministry of Education,Department of Chemical Engineering,Tsinghua University,Beijing 100084,China
  • Received:2020-08-16 Online:2021-02-10 Published:2020-11-19
  • Contact: ZHANG Rufan E-mail:zhangrufan@tsinghua.edu.cn
  • Supported by:
    ? Supported by the National Natural Science Foundation of China(51872156)

Abstract:

Two-dimensional metal-organic frameworks(MOFs) have attracted extensive attention due to their extraordinary merits such as high specific surface area, porous structure and abundant active sites, thus showing great potential in the field of electrocatalysis. Much progress has been made in their controlled synthesis and the modulation of their electrocatalytic performance, which reveals the crucial role of related resear-ches in the development of high-performance electrocatalysts. Top-down and bottom-up synthetic strategies of two-dimensional MOFs and typical synthetic methods of two-dimensional MOF derivatives are reviewed. The modulation strategies of the electrocatalytic performance of two-dimensional MOFs at various scales are summarized, and the electrocatalytic applications of these synthetic methods and modulation strategies are introduced. At last, the challenges and development directions for this area are also discussed.

Key words: Metal-organic framework, Electrocatalysis, Synthetic method, Performance modulation

CLC Number: 

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