Chem. J. Chinese Universities ›› 2018, Vol. 39 ›› Issue (7): 1524.doi: 10.7503/cjcu20170728
• Physical Chemistry • Previous Articles Next Articles
Received:
2017-11-13
Online:
2018-07-10
Published:
2018-06-08
Contact:
HE Xingquan
E-mail:hexingquan@hotmail.com
Supported by:
CLC Number:
TrendMD:
WANG Xiuli, HE Xingquan. Electrocatalytic Performance of Fe9S10 Nanoparticles Loaded Nitrogen and Sulphur Codoped Porous Carbon for Oxygen Reduction Reaction†[J]. Chem. J. Chinese Universities, 2018, 39(7): 1524.
Sample | Surface area/(m2·g-1) | Pore volume, V/(cm3·g-1) | Pore diameter, D/nm |
---|---|---|---|
Fe9S10/NSPC-700 | 208.1 | 0.55 | 10.60 |
Fe9S10/NSPC-800 | 331.3 | 0.68 | 8.24 |
Fe9S10/NSPC-900 | 398.9 | 1.64 | 16.48 |
Fe9S10/NSPC-1000 | 187.4 | 0.44 | 9.40 |
Fe9S10/NSC-900 | 261.9 | 0.65 | 9.96 |
Table 1 Structural parameters of different catalysts
Sample | Surface area/(m2·g-1) | Pore volume, V/(cm3·g-1) | Pore diameter, D/nm |
---|---|---|---|
Fe9S10/NSPC-700 | 208.1 | 0.55 | 10.60 |
Fe9S10/NSPC-800 | 331.3 | 0.68 | 8.24 |
Fe9S10/NSPC-900 | 398.9 | 1.64 | 16.48 |
Fe9S10/NSPC-1000 | 187.4 | 0.44 | 9.40 |
Fe9S10/NSC-900 | 261.9 | 0.65 | 9.96 |
Fig.7 CV curves of Fe9S10/NSPC-900 in N2, O2 saturated 0.1 mol/L KOH at a scan rate of 100 mV/s(A), LSV curves of Fe9S10/NSPC-900 at different rotation in O2 saturated 0.1 mol/L KOH with a scan rate of 10 mV/s(B), LSV polarization curves of Fe9S10/NSPC-T(C) and Fe9S10/NSC-900, Fe9S10/NSPC-900, NSPC-900 and Pt/C(D)
Fig.9 Rotating ring disk electrode(RRDE) measurements of Fe9S10/NSPC-900(a) and Pt/C(b) in 0.1 mol/L KOH(A), peroxide percentage and electron transfer number(inset) of Fe9S10/NSPC-900(a) and Pt/C(b) at different potentials(B)
Fig.10 Chronoamperometric curves of Fe9S10/NSPC-900(a) and Pt/C(b) in 0.1 mol/L KOH solution saturated with O2 at a rotation speed of 1600 r/min(A) and chronoamperometric response for ORR on Fe9S10/NSPC-900(a) and Pt/C(b) with the scan rate of 10 mV/s in 0.1 mol/L KOH solution saturated with O2 with 3 mol/L methanol added after 300 s(B)
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