新型CO2智能响应材料的研究进展

doi:10.7503/cjcu20141024

摘要/Abstract

摘要：

CO₂智能响应材料在受到CO₂刺激时, 材料自身物理结构或化学性质发生可逆转变. 本文根据对CO₂响应基团的不同, 将CO₂智能响应材料分成基于胺基基团和基于脒基基团的两大类, 分别对其制备方法和应用进行了综述, 并对CO₂智能响应材料的发展进行了展望.

Abstract:

Intelligent CO₂-responsive materials were kinds of new materials of which the physical structures or chemical properties will reversibly change when they were triggered by CO₂.These novel CO₂-responsive materials attracted wide attentions of scientists due to their characteristic CO₂-responsive mechanism and highly efficient transitional properties. In this review, the preparation methods and their application of the recent CO₂-responsive materials based on amino groups and amidine groups were reviewed, respectively. Meanwhile, the development prospect of the novel CO₂-responsive materials was also discussed.

Key words: Carbon dioxide, Intelligent responsive material, Amino, Amidine

中图分类号:

O631

TrendMD:

田彤, 李景辉, 王耀. 新型CO₂智能响应材料的研究进展. 高等学校化学学报, 2015, 36(3): 399.

TIAN Tong, LI Jinghui, WANG Yao. Research Progress of Intelligent CO₂-Responsive Materials^†. Chem. J. Chinese Universities, 2015, 36(3): 399.

图/表 20

Fig.1 Sorts of CO2 intelligent responsive materials[27]

Fig.2 Chemical principles governing CO2-air switchable wormlike micelles[35]

Fig.3 Schematic of protein capture and release using CO2-responsive polymer brushes[36]

Fig.4 Innovative nano-layered PEI/PSS solid sorbents for CO2 capture[38]

Fig.5 Mechanism of CO2 chemical sensing using polymer-coated carbon nanotube and its response of the carbon nanotube sensor to CO2 gas[39]

Fig.6 Schematic illustration of the CO2 responsive switchable surfactants[41]

Fig.7 Switching a solute’s partitioning behaviour[41]

Fig.8 Reaction of N,N-dimethyl-N'-(pyren-1-ylmethyl)acetimidamide with CO2 and water to create N,N-dimethyl-N'-(pyren-1-ylmethyl)acetamidinium bicarbonate salt[50]

Fig.9 Controlled dispersion and aggregation of SWNTs with a CO2-responsive dispersant[51]

Fig.10 Synthesis strategy of amidine-based polymer(A) and its reaction with CO2 and water(B) (B1) Amidine-based polymer in water after treatment with CO2; (B2) after treatment with N2 at 60 ℃ for 15 min; (B3) after treatment with CO2 at 60 ℃ again[52].

Fig.11 Schematic illustration of the dispersion of SWNTs by p-AP12 and their response to the stimulus of CO2 in water[53]

Fig.12 Phase behaviour of a mixture of water and an SHS(switchable-hydrophilicity solvent)[55]

Fig.13 Process of SHS used to extract soybean oil from soybean flakes without a distillation step[55] The dashed lines indicate the recycling of the solvent and the aqueous phase.

Fig.14 CO2-responsive switching of the NADPA SAM[56] (A) A photographic image of the water drop profile on a NADPA modified surface before(left) and after(right) the stimuli of dissolued CO2; (B) a schematic diagram of stimuliinduced transition of surface wettability; (C) changes of chemical structure of amidine; (D) reversible switching of water contact angles; (E) schematic illustration of selective adsorption of oleylamine- and citrate-capped Au NPs on the NADPA surface in response to dissolued CO2 stimuli.

Fig.15 Gas-switchable amidine-containing triblock copolymer EAS(top) and representation of its CO2-driven controlled self-assembly and shape transformation behaviour(bottom)[59]

Fig.16 Optical sensing scheme for carbon dioxide using a solvatochromic probe[66]

Fig.17 Schematic illustration of the amidine-based fluorescent chemosensor[67]

Fig.18 Chemical molecular structures of the PS-b-PEO and guest molecule M(A) and schematic of fabrication of PS-b-PEO/M membrane and an ideal model proposed for the nanostructured membrane(B)[72]

Fig.19 Reversible CO2 capture by HAMs[76] (A) The chemical structures of the HAMs; (B) the carbonation and decarbonation reactions of the HAMs.

Fig.20 Classification of new intelligent carbon dioxide responsive material and its application

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新型CO₂智能响应材料的研究进展

Research Progress of Intelligent CO₂-Responsive Materials^†

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