Chem. J. Chinese Universities ›› 2018, Vol. 39 ›› Issue (12): 2774.doi: 10.7503/cjcu20180496
• Polymer Chemistry • Previous Articles Next Articles
LI Xun1,2, XUE Yurui1, SONG Yu2,*(), ZHANG Wenke1
Received:
2018-07-11
Online:
2018-10-26
Published:
2018-10-26
Contact:
SONG Yu
E-mail:songyu16@jlu.edu.cn
Supported by:
CLC Number:
TrendMD:
LI Xun,XUE Yurui,SONG Yu,ZHANG Wenke. Coordinate Interaction Between Monosulfide and Au Surfaces†[J]. Chem. J. Chinese Universities, 2018, 39(12): 2774.
Fig.1 Histograms of the rupture forces of isolated single monosulfide from oxidized(red) and reduced(blue) gold surfaces, respectively(A) and representative force-extension curves obtained from SMFS experiments, for clarity those force curves were offset from trace to trace by 600 pN along the y-axis(B)
Scheme 3 Schematic drawing of the rupturing of isolated single 2-(ethylthio)ethylamine-gold contacts from the oxidized gold surfaces(step Ⅰ) and same AFM tip employed in(step Ⅰ) brought into contact with the sulphydryl-terminated silicon surfaces(step Ⅱ)
Fig.4 XPS spectra of bare gold and SAMs of 2-(ethylthio)ethylamine on oxidized(solid red trace) and reduced(dashed blue trace) gold surfaces(A) Au4f;(B) S2p.
Fig.5 Histograms of the rupture forces of individual sulfide-gold contacts obtained from SAMs of 2-(ethylthio)ethylamine on oxidized(red) and reduced(blue) gold surfaces in 1,4-dioxane
Fig.6 Comparison of the unbinding forces of individual thioether molecule from SAMs of 2-(ethylthio)ethylamine on reduced gold surfaces in PBS(pH=8.0) and 1,4-dioxane conditions
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