Optical Properties and Applications of Halide-perovskite Nanocrystals†

doi:10.7503/cjcu20170788

Abstract

Abstract:

Halide perovskite-type ABX₃ nanocrystals mainly including the optical properties and applications of all-inorganic ABX₃ nanocrystals were reviewed. First of all, the two preparation methods of atmospheric pressure, solvent heating and ion-exchange process for all-inorganic nanocrystals are reported; then, the optical properties of their absorption and photoluminescence are elaborated in detail; finally, their applications in light emitting diode(LED) and solar cell are emphasically elucidated, and also involving in the fields of laser, photodetector and photocatalysis. In the recent future, the halide perovskite nanocrystals will also definitely exhibit other potential applications owing to the excellent optical and electrical properties.

Key words: Perovskite-phase, Halide, Nanocrystals, Optical property, Photoluminescence

CLC Number:

O614
O646

TrendMD:

JI Tianhao, TIAN Yanqing. Optical Properties and Applications of Halide-perovskite Nanocrystals^†[J]. Chem. J. Chinese Universities, 2018, 39(6): 1113.

Figures/Tables 4

Fig.1 Optical absorption spectra of CsPbX3 nanocrystals[28]Copyright from the American Chemical Society.

Fig.2 Effects of halide ions on the band gap and PLQY in CsPbX3[29](A) PL spectra of CsPb(Br∶X)3(X=Cl, I) NCs prepared by anion exchange from CsPbBr3 NCs; (B) PL calibration curves: a targeted emission energy could be obtained by adding a precise amount of halide precursor to a crude solution of CsPbBr3 NCs; (C) PLQY recorded on the exchanged NCs(dots) as well as the directly synthesized NCs(stars). Copyright from the American Chemical Society.

Fig.3 LED structure with 6.27% of EQE value[60] Copyright from the John Wiley and Sons.

Fig.4 Chemical structures of spiro-OMeTAD, HTM1 and HTM2(A) and normalized UV-Vis absorption spectra of HTM1, HTM2 and spiro-OMeTAD in THF solution(B)[64]Copyright from the Royal Society of Chemistry.

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