基于离子液体的绿色电子器件

doi:10.7503/cjcu20190634

摘要/Abstract

摘要：

基于离子液体的绿色液体电子器件可回收性强, 且具备柔性、自修复性、可重塑与可重构性等性能, 拓宽了液体电子器件的应用范围, 为绿色环保的多功能电子器件的开发提供了新途径. 本文围绕离子液体基的电子器件进行了总结, 并阐述了该类器件广阔的应用前景.

关键词: 绿色电子器件, 离子液体, 可回收性

Abstract:

Our group has devoted to using ionic liquids as sensing materials to fabricate green electronic devices. This particular class of sensing liquids possesses intrinsic advantages of excellent recyclability, flexibility, self-healing property, remoldability and reconfigurability. There are still some challenges of synthesizing kinds of liquid electronic materials and fabricating complex integrated circuits. The breakthrough of these problems will broaden the application range of green electronic devices and provide an effective method to exploit multi-function green electronic devices. This review mainly pays attention to the development of electronic devices based on ionic liquids and perdict the enornous potential applications of this devices.

Key words: Green electronic device, Ionic liquid, Recyclability

中图分类号:

TrendMD:

高乃伟, 马强, 贺泳霖, 王亚培. 基于离子液体的绿色电子器件. 高等学校化学学报, 2020, 41(5): 901.

GAO Naiwei, MA Qiang, HE Yonglin, WANG Yapei. Green Electronic Devices Based on Ionic Liquids ^†. Chem. J. Chinese Universities, 2020, 41(5): 901.

图/表 5

Fig.1 Liquid electronic materials and healthy monitor of liquid temperature sensors[24,27,28] (A) Optical image of flexible temperature sensor[24]. (B) The measurement of resistance stability of flexible temperature sensor at different stress[24]. (C—E) Flexible ionic liquid-based temperature sensor and the monitoring of body temperature[24]. Copyright 2015, John Wiley and Sons. (F) Optical image of self-healing temperature sensor[27]. (G) The electrical response of different ionic liquids against temperature change[27]. Copyright 2015, John Wiley and Sons. (H) Measurement of periodic temperature change of female volunteer by the CaCl2/EG-based temperature sensor[28]. Copyright 2018, American Chemical Society.

Fig.2 Mechanism and measurement of liquid strain sensors based on ionic liquids[24] (A) Schematic illustration of the sensing principle of liquid strain sensors via partially filling [OMIm]Ac into a PDMS sponge. (B) the relationship between volume fraction of ionic liquid and the conductivity change at a given pressure of 0.5 N. (C) Pressure sensing performance of PDMS sponge with different crosslinking degrees, the pressure ranges from 0.25 to 3.00 N with an interval of 0.25 N. (D) Pressure sensing measurements of PDMS sponge with crosslinking degree of 20:1 at different pressure forces. Copyright 2015, John Wiley and Sons.

Fig.3 Near infrared response measurement of liquid NIR sensors based on ionic liquids[24,37] (A) Structure of the flexible NIR sensor based on PPyNPs@[OMIm][Ac][24]. (B) NIR sensing of flexible NIR sensor doping with different mass fraction of PPy NPs at different NIR power[24]. Copyright 2015, John Wiley and Sons. (C) Mechanism of light sensing by poly-[Py-Cn-MIm]Br on the basis of photothermal conversion[37]. (D) Optical image of multi-channel light sensor[37]. (E, F) IR image and electrical responses of flexible light sensors[37]. Copyright 2019, American Chemical Society.

Fig.4 Mechanicalmodel of liquid sensors based on ionic liquids confined by straight-shape capillary channel[27] (A), (B) The mechanical analysis of ionic liquids filled in a straight-shape capillary channel. (C), (D) Optical images of a vertically placed microchannel filled with [OMIm]PF6. The diameters of microchannel are 1.615 mm(C) and 0.709 mm(D), respectively. Copyright 2015, John Wiley and Sons.

Fig.5 Preparation and repairable measurement of crystal-confined freestanding ionic liquids[41] (A) Preparation of crystal-confined ionic liquids as a complex of [OMIm]PF6 and [OMIm]AzoO through a super-saturated solution cooling method. (B) A mathematical model to demonstrate the pinning capillary effect by [OMIm]AzoO crystals. (C) Optical images of self-healing robotic arms made of crystal-confined ionic liquids. (D) Repairable measurement through the process of cutting and healing of the robotic arm at different status. Copyright 2019, Springer Nature.

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