Chem. J. Chinese Universities ›› 2019, Vol. 40 ›› Issue (10): 2170.doi: 10.7503/cjcu20190226
• Physical Chemistry • Previous Articles Next Articles
YIN Mengxin,LIU Dongsheng,ZHAO Dongyue,DING Tong,TIAN Ye,LI Xingang()
Received:
2019-04-18
Online:
2019-10-08
Published:
2019-08-20
Contact:
LI Xingang
E-mail:xingang_li@tju.edu.cn
Supported by:
TrendMD:
YIN Mengxin,LIU Dongsheng,ZHAO Dongyue,DING Tong,TIAN Ye,LI Xingang. Effect of Copper Doping on Lean NOx Trap Performance of Pt/Ba/CuxMg1-xAl2O4 Catalysts at High Temperatures [J]. Chem. J. Chinese Universities, 2019, 40(10): 2170.
Support | SBET/(m2·g-1) | Pore volume/(cm3·g-1) | Pore diameter/nm |
---|---|---|---|
MgAl2O4 | 162.2 | 0.4 | 10.6 |
Cu0.1Mg0.9Al2O4 | 186.9 | 0.6 | 12.1 |
Cu0.3Mg0.7Al2O4 | 227.0 | 0.6 | 10.2 |
Support | SBET/(m2·g-1) | Pore volume/(cm3·g-1) | Pore diameter/nm |
---|---|---|---|
MgAl2O4 | 162.2 | 0.4 | 10.6 |
Cu0.1Mg0.9Al2O4 | 186.9 | 0.6 | 12.1 |
Cu0.3Mg0.7Al2O4 | 227.0 | 0.6 | 10.2 |
Catalyst | Oads/Olatt | Molar fraction of Pt(%) |
---|---|---|
Pt/Ba/MgAl2O4 | 0.14 | 1.1 |
Pt/Ba/Cu0.1Mg0.9Al2O4 | 0.21 | 1.3 |
Pt/Ba/Cu0.3Mg0.7Al2O4 | 0.17 | 1.5 |
Catalyst | Oads/Olatt | Molar fraction of Pt(%) |
---|---|---|
Pt/Ba/MgAl2O4 | 0.14 | 1.1 |
Pt/Ba/Cu0.1Mg0.9Al2O4 | 0.21 | 1.3 |
Pt/Ba/Cu0.3Mg0.7Al2O4 | 0.17 | 1.5 |
Catalyst | NO to NO2 conversion(%) | NOx reduction efficiency(%) | NSC/(mmol·g-1) | NRP(%) |
---|---|---|---|---|
Pt/Ba/MgAl2O4 | 48.0 | 87.0 | 0.58 | 72.9 |
Pt/Ba/Cu0.1Mg0.9Al2O4 | 53.6 | 92.1 | 0.67 | 89.7 |
Pt/Ba/Cu0.3Mg0.7Al2O4 | 60.9 | 88.6 | 0.65 | 82.9 |
Catalyst | NO to NO2 conversion(%) | NOx reduction efficiency(%) | NSC/(mmol·g-1) | NRP(%) |
---|---|---|---|---|
Pt/Ba/MgAl2O4 | 48.0 | 87.0 | 0.58 | 72.9 |
Pt/Ba/Cu0.1Mg0.9Al2O4 | 53.6 | 92.1 | 0.67 | 89.7 |
Pt/Ba/Cu0.3Mg0.7Al2O4 | 60.9 | 88.6 | 0.65 | 82.9 |
Fig.6 NOx-TPD profiles of the catalysts(A) and enlarged view of the red rectangle area in profile (A)(B) a. Pt/Ba/MgAl2O4; b. Pt/Ba/Cu0.1Mg0.9Al2O4; c. Pt/Ba/Cu0.3Mg0.7Al2O4. The dotted line is the trend of temperature over time.
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