高等学校化学学报 ›› 2020, Vol. 41 ›› Issue (12): 2638.doi: 10.7503/cjcu20200396
• 庆祝《高等学校化学学报》复刊40周年专栏 • 上一篇 下一篇
收稿日期:
2020-06-29
出版日期:
2020-12-10
发布日期:
2020-12-09
通讯作者:
夏帆
E-mail:xiafan@cug.edu.cn
基金资助:
WANG Dagui, CHEN Yajie, JIAN Qi, GAO Pengcheng, XIA Fan()
Received:
2020-06-29
Online:
2020-12-10
Published:
2020-12-09
Contact:
XIA Fan
E-mail:xiafan@cug.edu.cn
Supported by:
摘要:
构筑聚合物抗污涂层表面是解决生物污损的有效策略. 聚合物具有耐酸碱性和易于功能化及表面修饰等优点, 聚合物抗污涂层在降低生物污损对材料的影响和减少经济损失中发挥着重要作用. 本文综合评述了聚合物抗污涂层的各种研究策略和研究进展, 介绍了相关新型聚合物抗污涂层的成果, 并展望了该领域面临的挑战.
中图分类号:
TrendMD:
王大贵, 陈雅捷, 简琦, 高鹏程, 夏帆. 聚合物抗污涂层的研究进展. 高等学校化学学报, 2020, 41(12): 2638.
WANG Dagui, CHEN Yajie, JIAN Qi, GAO Pengcheng, XIA Fan. Research Advance of Polymer Anti-fouling Coatings. Chem. J. Chinese Universities, 2020, 41(12): 2638.
Fig.1 Schematic of biofilm development(A)[14] and different kinds of biological fouling from microscales to macroscales(B)[27](A) Copyright 2014, Elsevier; (B) Copyright 2013, Springer Nature.
Fig.3 Preparation and performance tests of coatings[38](A) Schematic diagram of the coating process(1 to 5), the coating structure(5), the structure of a partially worn coating(6), and AFM image of a PU coating containing 25%(mass fraction) of fluorine(7); (B) anti smudge properties of P3?modified PU films containing 6.6%(mass fraction) fluorine.Copyright 2015, Wiley?VCH.
Fig.4 Preparation and anti?adhesion tests of TP/LP surfaces[39](A) Schematic of blood repellency on TLP surfaces; (B) surfaces without TP or LP(?TP/?LP; control) show adhesion of a blood droplet, scale bars, 1 cm.Copyright 2014, Springer Nature.
Fig.5 Schematic of synthesis of PSBMA brushes via Si?ATRP polymerization on Si substrate(A) and schematic illustration of the ice adhesion strength measurement and the results(B)[50]Copyright 2019, American Chemical Society.
Fig.6 Preparation and oil?water separation tests of PMPC coatings[51](A) Schematic illustration of grafting PMPC onto a gold substrate; (B) photos of stainless steel meshes coated without(left) and with(right) PMPC coatings in oil and test of lifting of petroleum out from a petroleum?water mixture.Copyright 2015, American Chemical Society.
Fig.7 Preparation and antimicrobial tests of each surfaces[61](A) Schematic illustration of preparation of the PMOXA/PDA film and also the representation of the structure of the polymeric film on the surface; (B) antimicrobial activities of each membrane against S. aureus.Copyright 2013, American Chemical Society.
Fig.8 Preparation and protein adsorption of polymer film[62](A) Synthetic route for linear PMOXA?OH and multiarm star copolymer PEI?g?PMOXA, and schematic illustration of preparation of the PMOXA/PDA film.(B) The amount of five di?erent types of proteins adsorbed on the gold surfaces before and after modification with polymers.Copyright 2015, Royal Society Chemistry.
Fig.9 Preparation and applied tests of FLIPS[78](A) A diagram showing the concept of FLIPS. Left, two topographical states of a ferrofluid spreading on an unstructured surface; right, top?view photo of FLIPS under magnetic field, region (1) exhibits micro?topography shaped by the structured substrate; region (2) exhibits a flat surface; and region (3) exhibits the macro?topographical protuberance.(B―D) Adhesion, pumping and biofilm removal(application of FLIPS at centimetre scale), respectively.Copyright 2018, Springer Nature.
Fig.10 Preparation and anti?fouling test of TO coatings[79](A) Schematic representation of the preparation procedure based on electrodeposition of a rough tungsten oxide(TO) ?lm on steel; (B) the samples just before(top panels) and after(bottom panels) being removed from the culture and dried: TO?SLIPS, TO?SHS and untreated stainless?steel control.Copyright 2015, Springer Nature.
Fig.11 Preparation and anti?fouling tests of water?like polymers coating(A) Preparation of the omniphobic Me2Si(OMe)2 derived SOCAL?PDMS coating[92]; (B) topographic image of the SOCAL coa?ting on a silicon wafer[92]; (C) formation of the SOCAL?PDMS coating by rapid acid?catalyzed polycondensation on a dimethyldimethoxysilane on a substrate surface[92]; (D) schematic diagram showing the structures of the reactive oil?repellent surface; (E) scheme of fabricating the reactive oil?repellent surface[93]; (F) images showing the mobility of a dyed chloroform droplet on treated and untreated regions of a glass display[93]; (G) ink?resistant test by an oil?based permanent ink marker on treated and untreated glass slides[93].(A―C) Copyright 2016, Wiley?VCH; (D―G) Copyright 2017, American Chemical Society.
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