Chem. J. Chinese Universities ›› 2019, Vol. 40 ›› Issue (4): 685.doi: 10.7503/cjcu20180741
• Analytical Chemistry • Previous Articles Next Articles
WU Xuemei1, WEI Jie1, XU Hongping2, ZUO Lingxia2, SHAN Xiaoyan2, YAO Huiqin1,2,*(), ZHENG Zhixiang3
Received:
2018-11-01
Online:
2019-04-03
Published:
2019-01-09
Contact:
YAO Huiqin
E-mail:huiqin_yao@163.com
Supported by:
TrendMD:
WU Xuemei,WEI Jie,XU Hongping,ZUO Lingxia,SHAN Xiaoyan,YAO Huiqin,ZHENG Zhixiang. Switchable Electrochemical Behavior of Matrine and Sophoridine at Multi-stimuli Responsive Hydrogel Film Electrode and Construction of Logic Gate†[J]. Chem. J. Chinese Universities, 2019, 40(4): 685.
Fig.1 CVs of 0.01 mol/L MT(A) and SR(B) at different pH values and effects of pH value on the Ipa and oxidation peak potential(Epa) of MT(C) and SR(D)pH: a. 4.0; b. 5.0; c. 6.0; d. 7.0; e. 8.0; f. 9.0.
Fig.3 CVs curves of 0.01 mol/L SR at 0.05 V/s in pH=9.0 NaCl solution without Na2SO4 for PNIPAM films at different temperatures(A), influence of solution temperature on Ipa of SR(a) and MT(b) in pH=9.0 NaCl solution(B) and variation of Ipa of 0.01 mol/L SR at 0.05 V/s in pH=9.0 NaCl solution with immersion time at temperature switched between 25 ℃ and 40 ℃ for the same PNIPAM films(C)(A) Temperature/℃: a. 25; b. 27; c. 29; d. 31; e. 33; f. 35; g. 37; h. 39; i. 40.
Fig.4 SEM top-view images of PNIPAM hydrogel films on GC surface after treated with pH=9.0 NaCl solutions(A) At 25 ℃; (B) at 40 ℃; (C) containing 0.45 mol/L Na2SO4 at 25 ℃; (D) containing 20%(volume fraction) methanol at 25 ℃.
Fig.5 CVs curves of 0.01 mol/L MT at 0.05 V/s in pH=9.0 NaCl solutions containing 0(a), 0.05(b), 0.10(c), 0.15(d), 0.20(e), 0.25(f), 0.30(g), 0.35(h), 0.40(i) and 0.45 mol/L(j) Na2SO4 for PNIPAM films at 25 ℃(A), variation of Ipa of 0.01 mol/L MT with immersion time containing 0 and 0.45 mol/L Na2SO4(B) and dependence of Ipa of 0.01 mol/L MT at 0.05 V/s in pH=9.0 NaCl solutions at 25 ℃ on Na2SO4(a), MgSO4(b), NaCl(c) and NaNO3(d) for PNIPAM films(C)
Fig.6 Influence of methanol volume fraction(0—40%) in water/methanol mixture solvent on Ipa of MT in pH=9.0 solutions for PNIPAM films at 25 ℃(A), variation of Ipa with immersion time in solutions containing 0() and 20%() methanol(B) and CVs of 0.01 mol/L MT containing 0(a) and 20%(b) methanol at bare GC electrodes(scan rate: 0.05 V/s)(C)
Fig.7 Ipa(CVs) obtained after application of eight combinations of the three input signalsThe dashed lines show the threshold values separating output signals. Inset: logic circuit for the 3-input/2-output logic gate system(input A=temperature, input B=Na2SO4, input C=methanol).
Input A(Temperature) | 1 | 1 | 1 | 0 | 1 | 0 | 0 | 0 |
---|---|---|---|---|---|---|---|---|
Input B(S | 1 | 1 | 0 | 1 | 0 | 1 | 0 | 0 |
Input C(Methanol) | 1 | 0 | 1 | 1 | 0 | 0 | 1 | 0 |
Output(Ipa) | 1 | 0 | 0 | 0 | 0 | 0 | 0 | 0 |
Table 1 Truth values of 3-input/2-output logic gate system
Input A(Temperature) | 1 | 1 | 1 | 0 | 1 | 0 | 0 | 0 |
---|---|---|---|---|---|---|---|---|
Input B(S | 1 | 1 | 0 | 1 | 0 | 1 | 0 | 0 |
Input C(Methanol) | 1 | 0 | 1 | 1 | 0 | 0 | 1 | 0 |
Output(Ipa) | 1 | 0 | 0 | 0 | 0 | 0 | 0 | 0 |
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