Chem. J. Chinese Universities ›› 2015, Vol. 36 ›› Issue (7): 1246.doi: 10.7503/cjcu20141082
• Articles: Inorganic Chemistry • Previous Articles Next Articles
ZHANG Xingxing, WU Chengzhang*(), ZHOU Jianfang, YANG Gonghui, LIU Yinhe, ZHANG Yuwen, DING Weizhong
Received:
2014-12-08
Online:
2015-07-10
Published:
2015-06-12
Contact:
WU Chengzhang
E-mail:wucz@shu.edu.cn
Supported by:
CLC Number:
TrendMD:
ZHANG Xingxing, WU Chengzhang, ZHOU Jianfang, YANG Gonghui, LIU Yinhe, ZHANG Yuwen, DING Weizhong. Oxygen Permeation Property and Structural Stabiltiy of La-doped BaCo0.88Nb0.12O3-δ Membranes in CO2 Atmosphere†[J]. Chem. J. Chinese Universities, 2015, 36(7): 1246.
Fig.1 XRD patterns(A) and (110) reflection peaks(B) of as-synthesized BLCN-x powdersa. BCN; b. BLCN-0.1; c. BLCN-0.2;d. BLCN-0.3; e. BLCN-0.5; f. LCN.
Membrane | Lattice parameter/nm | ABE/(kJ·mol-1) | Tolerance factor(Co4+/Co3+) | Activation energy/(kJ·mol-1) |
---|---|---|---|---|
BCN | 0.408 | -279.1 | 1.084/1.091 | 35.8, 132.7 |
BCLN-0.1 | 0.404 | -285.2 | 1.076/1.083 | 65.1 |
BLCN-0.2 | 0.401 | -291.2 | 1.067/1.074 | 67.0 |
BLCN-0.3 | 0.396 | -297.3 | 1.058/1.065 | 70.1 |
BLCN-0.5 | 0.391 | -309.3 | 1.041/1.048 | 56.5 |
LCN | 0.382 | -339.2 | 0.998/1.004 | 36.2 |
Table 1 Calculated lattice parameters, tolerance factor, activation energy of the oxygen permeability, and average metal-oxygen bond energy(ABE) for BLCN-x membranes
Membrane | Lattice parameter/nm | ABE/(kJ·mol-1) | Tolerance factor(Co4+/Co3+) | Activation energy/(kJ·mol-1) |
---|---|---|---|---|
BCN | 0.408 | -279.1 | 1.084/1.091 | 35.8, 132.7 |
BCLN-0.1 | 0.404 | -285.2 | 1.076/1.083 | 65.1 |
BLCN-0.2 | 0.401 | -291.2 | 1.067/1.074 | 67.0 |
BLCN-0.3 | 0.396 | -297.3 | 1.058/1.065 | 70.1 |
BLCN-0.5 | 0.391 | -309.3 | 1.041/1.048 | 56.5 |
LCN | 0.382 | -339.2 | 0.998/1.004 | 36.2 |
Fig.4 SEM images of BLCN-x membranes after calcining at 850 ℃ for 5 h under pure CO2 atmosphere(A) BCN; (B) BLCN-0.1; (C) BLCN-0.2; (D) BLCN-0.3; (E) BLCN-0.5; (F) LCN.
Fig.6 CO2 TPD-MS spectra of BLCN-x powders calcined at 850 ℃ for 5 h under pure CO2 atmospherea. BCN; b. BLCN-0.1; c. BLCN-0.2; d. BLCN-0.3; e. BLCN-0.5. Inset is the magnified TPD-MS spectra of BLCN-0.3 and BLCN-0.5.
Fig.7 Temperature dependence of oxygen permeable flues through BLCN-x membranes(A) and related Arrhenius plots(B)a. BCN; b. BLCN-0.1; c. BLCN-0.2; d. BLCN-0.3; e. BLCN-0.5; f. LCN.
Fig.8 Oxygen permeation flues of BLCN-x membrane swept by pure CO2 at 850 ℃Thickness of membrane: 0.5 mm;air flow rate: 110 mL/min;CO2 flow rate: 80 mL/min.
Fig.9 XRD patterns of BLCN-x membranes after oxygen permeation for 10 h at 850 ℃ under pure CO2 atmospherea. BCN; b. BLCN-0.1; c. BLCN-0.2;d. BLCN-0.3; e. BLCN-0.5; f. LCN.
[1] | Haszeldine R. S., Science, 2009, 325, 1647—1652 |
[2] | Kvamsdal H. M., Jorda K. L., Bolland O., Energy, 2007, 32, 10—24 |
[3] | Chiesa P., Kreutz T. G., Lozza G. G., J. Engin. Gas Turb. Power, 2007, 129, 123—134 |
[4] | Leo A., Liu S. M., Costa J. C. D., Int. J. Greenh. Gas. Con., 2009, 3, 357—367 |
[5] | Teraoka Y., Zhang H. M., Yamazoe N., Chem. Lett., 1985, 9, 1367—1370 |
[6] | Zhang P., Guan G., Khaerudini D. S., Hao X., Han M., Kasai Y., Sasagawa K., Abudula A., J. Power Sources, 2014, 248, 163—171 |
[7] | Li H. B., Zhu X. F., Liu Y., Wang W. P., Yang W. S., J. Membr. Sci., 2014, 462, 170—177 |
[8] | Shao Z. P., Dong H., Xiong G. X., Gong Y., Yang W. S., J. Membr. Sci., 2001, 183, 181—192 |
[9] | Luo H.X., Jiang H. Q., Klande T., Cao Z. W., Liang F. Y., Wang H. H., Caro J., Chem. Mater., 2012, 24, 2148—2154 |
[10] | Harada M., Domen K., Hara M., Tatsumi T., Chem. Lett., 2006, 35, 1326—1327 |
[11] | Benson S. J., Waller D., Kilner J. A., J. Electrochem. Soc., 1999, 146, 1305—1309 |
[12] | Yi J. X., Schroeder M., Weirich T., Mayer J., Chem. Mater., 2010, 22, 6246—6253 |
[13] | Arnold M., Wang H. H., Feldhoff A., J. Membr. Sci., 2007, 293, 44—52 |
[14] | Wu C. Z., Wang H., Zhang X. X., Zhang Y. W., Ding W. Z., Sun C. H., J. Energy Chem., 2014, 23, 575—581 |
[15] | Zeng Q., Zuo Y., Fan C., Chen C., J. Membr. Sci., 2009, 335, 140—144 |
[16] | Yi J. X., Brendt J., Schroeder M., Martin M., J. Membr. Sci., 2012, 387, 17—23 |
[17] | Zhu X. F., Liu H. Y., Cong Y., Yang W. S., Chem. Commun., 2012, 48, 251—253 |
[18] | Luo H., Efimov K., Jiang H., Feldhoff A., Wang H., Caro J., Angew. Chem. Int. Ed., 2011, 50, 759—763 |
[19] | Geng Z., Ding W. Z., Wang H. H., Wu C. Z., Shen P. J., Meng X. Y., Gai Y. Q., Ji F. T., J. Membr. Sci., 2012, 403, 140—145 |
[20] | Zhang Y. W., Su K., Zeng F. L., Ding W. Z., Lu X. G., Int. J. Hydrogen Energy, 2013, 38, 8783—8789 |
[21] | Shen P. J., Ding W. Z., Zhang Y. W., Zhou Y. D., Yang Z. B., Qin G. L., Chem. J. Chinese Universities, 2009, 30(1), 152—158 |
(沈培俊, 丁伟中, 张玉文, 周宇鼎, 杨志彬, 秦国利. 高等学校化学学报,2009, 30(1), 152—158) | |
[22] | Meng X. Y., Ding W. Z., Jin R., Wang H., Gai Y. Q., Ji F. T., Ge Y., Xie D. Q., J. Membr. Sci., 2014, 450, 291—298 |
[23] | Liu X., Ding W. Z., Shen P. J., Liu J., Wang H. H., Geng Z., J. Shanghai University.(Natural Science Edition), 2011, 17(1), 7—12 |
(刘旭, 丁伟中, 沈培俊, 刘蛟, 王海海, 耿振.上海大学学报(自然科学版), 2011, 17(1), 7—12) | |
[24] | Gai Y. Q., Ding W. Z., Jin R., Meng X. Y., Ji F. T., Wang H., J. Funct. Mater., 2014, 5, 5045—5048 |
(盖永乾, 丁伟中, 金容, 孟星宇, 吉福堂, 王贺.功能材料, 2014, 5, 5045—5048) | |
[25] | Ramadass N., Mater. Sci. Eng., 1978, 36, 231—240 |
[26] | Zhu X. F., Cong Y., Yang W. S., Solid State Ionics, 2006, 177, 2917—2921 |
[27] | Sammells A. F., Cook R. L., White J. H., Osborne J. J., MacDuff R. C., Solid State Ionics, 1992, 52, 111—123 |
[1] | CHENG Qian, YANG Bolong, WU Wenyi, XIANG Zhonghua. S-doped Fe-N-C as Catalysts for Highly Reactive Oxygen Reduction Reactions [J]. Chem. J. Chinese Universities, 2022, 43(9): 20220341. |
[2] | JIA Yanggang, SHAO Xia, CHENG Jie, WANG Pengpeng, MAO Aiqin. Preparation and Lithium Storage Performance of Pseudocapacitance-controlled Perovskite High-entropy Oxide La(Co0.2Cr0.2Fe0.2Mn0.2Ni0.2)O3 Anode Materials [J]. Chem. J. Chinese Universities, 2022, 43(8): 20220157. |
[3] | SONG Youwei, AN Jiangwei, WANG Zheng, WANG Xuhui, QUAN Yanhong, REN Jun, ZHAO Jinxian. Effects of Ag,Zn,Pd-doping on Catalytic Performance of Copper Catalyst for Selective Hydrogenation of Dimethyl Oxalate [J]. Chem. J. Chinese Universities, 2022, 43(6): 20210842. |
[4] | SUN Xuefeng, RENAGUL Abdurahman, YANG Tongsheng, YANG Qianting. Synthesis and Luminescence Properties of Cr,In Co-doped Small Size MgGa2O4 Near-infrared Persistent Luminescence Nanoparticles [J]. Chem. J. Chinese Universities, 2022, 43(4): 20210850. |
[5] | WANG Zumin, MENG Cheng, YU Ranbo. Doping Regulation in Transition Metal Phosphides for Hydrogen Evolution Catalysts [J]. Chem. J. Chinese Universities, 2022, 43(11): 20220544. |
[6] | YUAN Meng, ZHAO Yingjie, WU Yuchen, JIANG Lei. Assembly of Perovskite Arrays and Multifunctional Detector Applications [J]. Chem. J. Chinese Universities, 2022, 43(11): 20220448. |
[7] | GAO Zhongnan, GUO Lihong, ZHAO Dongyue, LI Xingang. Effect of A Site-deficiency on the Structure and Catalytic Oxidation Activity of the La-Sr-Co-O Perovskite [J]. Chem. J. Chinese Universities, 2021, 42(9): 2869. |
[8] | HONG Yangyu, XING Hongzhu, BING Qiming, GAO Xuwen, QI Bin, CHEN Yakun, SU Tan, ZOU Bo. Synthesis and Fluorescence Properties of Novel Ce3+-doped Manganese Phosphite Open-framework Materials [J]. Chem. J. Chinese Universities, 2021, 42(9): 2725. |
[9] | WU Yaqiang, LIU Siming, JIN Shunjin, YAN Yongqing, WANG Zhao, CHEN Lihua, SU Baolian. Synthesis of Zn-Doped NiCoP Catalyst with Porous Double-layer Nanoarray Structure and Its Electrocatalytic Properties for Hydrogen Evolution [J]. Chem. J. Chinese Universities, 2021, 42(8): 2483. |
[10] | CHEN Mingsu, ZHANG Huiru, ZHANG Qi, LIU Jiaqin, WU Yucheng. First-principles Study on the Catalytic Effect of Co,P co-Doped MoS2 in Lithium-sulfur Batteries [J]. Chem. J. Chinese Universities, 2021, 42(8): 2540. |
[11] | YUE Shengli, WU Guangbao, LI Xing, LI Kang, HUANG Gaosheng, TANG Yi, ZHOU Huiqiong. Research Progress of Quasi-two-dimensional Perovskite Solar Cells [J]. Chem. J. Chinese Universities, 2021, 42(6): 1648. |
[12] | LI Yishan, GUO Liang, PENG Sifan, ZHANG Qingmao, ZHANG Yuhao, XU Shiqi. Cobalt Substitutions in Lanthanum Manganate Photocatalyst: First-principles and Visible-light Photocatalytic Ability Investigation [J]. Chem. J. Chinese Universities, 2021, 42(6): 1881. |
[13] | WANG Kunhua, YAO Jisong, YANG Junnan, SONG Yonghui, LIU Yuying, YAO Hongbin. Synthesis and Device Optimization of Highly Efficient Metal Halide Perovskite Light-emitting Diodes [J]. Chem. J. Chinese Universities, 2021, 42(5): 1464. |
[14] | DONG Luming, SU Yanyue, WANG Chunzheng, QIAO Yafei, CHEN Yajun, MA Haiyun. Synthesis of Micro- to Nano-scale Perovskite Calcium Hydroxytinate and Its Performance as a Flame Retardant in Epoxy Resin [J]. Chem. J. Chinese Universities, 2021, 42(3): 937. |
[15] | CHEN Xiaoyu, YU Ranbo. Research Progress on Doping of Molybdenum Disulfide and Hydrogen Evolution Reaction [J]. Chem. J. Chinese Universities, 2021, 42(2): 475. |
Viewed | ||||||
Full text |
|
|||||
Abstract |
|
|||||